Admittedly, I’ve never played Supervillains (which might change depending on what turns up under the ol’ Christmas Tree this year). Personally, I really like 2, but the original manages to capture the franchise’s tone and style perfectly while still being fun and LEGO-ish. 3 kinda sucks. At least relative to other LEGO games.
I’ve never played villains either but I loved flying around the city in 2. Seemed like every corner you turned had some surprise. In retrospect, it is like Arkham City with more than one character.
I like the DC Villains but I’ll always like Lego Batman 2 cause it’s the first and only Lego game I ever completed 100%. Does Lego Dimension count? That was a fun game also.